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04167nam a22005775i 4500 |
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978-3-030-54851-3 |
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DE-He213 |
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20211012191729.0 |
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cr nn 008mamaa |
| 008 - FIXED-LENGTH DATA ELEMENTS--GENERAL INFORMATION |
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200910s2020 sz | s |||| 0|eng d |
| 020 ## - INTERNATIONAL STANDARD BOOK NUMBER |
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| International Standard Book Number |
9783030548513 |
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978-3-030-54851-3 |
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10.1007/978-3-030-54851-3 |
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doi |
| 050 #4 - LIBRARY OF CONGRESS CALL NUMBER |
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QC170-197 |
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QC717.6-718.8 |
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PHM |
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bicssc |
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SCI074000 |
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bisacsh |
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PHM |
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thema |
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| Classification number |
539 |
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23 |
| 100 1# - MAIN ENTRY--PERSONAL NAME |
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| Personal name |
Liu, Lai Chung. |
| 245 10 - TITLE STATEMENT |
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| Title |
Chemistry in Action: Making Molecular Movies with Ultrafast Electron Diffraction and Data Science |
| Statement of responsibility, etc |
by Lai Chung Liu. |
| 250 ## - EDITION STATEMENT |
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| Edition statement |
1st ed. 2020. |
| 300 ## - PHYSICAL DESCRIPTION |
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| Extent |
XX, 239 p. 110 illus., 106 illus. in color. |
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online resource. |
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| Formatted contents note |
Chapter1: Introduction -- Chapter2: Methods: Experimental Techniques and Data Science -- Chapter3: Ultrafast Structural Dynamics of (EDO-TTF)2X -- Chapter4: Photocyclization Dynamics of Diarylethene -- Chapter5: Photoinduced Spin Crossover in Iron(II) Systems -- Chapter6: Future Work -- Chapter7: Conclusion. |
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| Topical term or geographic name as entry element |
Atoms. |
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Physics. |
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Chemistry, Physical and theoretical. |
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Analytical chemistry. |
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Crystallography. |
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Atomic, Molecular, Optical and Plasma Physics. |
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Theoretical and Computational Chemistry. |
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Analytical Chemistry. |
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Crystallography and Scattering Methods. |
| 710 2# - |
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SpringerLink (Online service) |
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| Uniform Resource Identifier |
https://doi.org/10.1007/978-3-030-54851-3 |
| 100 1# - MAIN ENTRY--PERSONAL NAME |
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author. |
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aut |
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http://id.loc.gov/vocabulary/relators/aut |
| 245 10 - TITLE STATEMENT |
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[electronic resource] / |
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Cham : |
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Springer International Publishing : |
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Imprint: Springer, |
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2020. |
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text |
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txt |
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rdacontent |
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computer |
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rdamedia |
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online resource |
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rdacarrier |
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text file |
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PDF |
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rda |
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Springer Theses, Recognizing Outstanding Ph.D. Research, |
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2190-5061 |
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The thesis provides the necessary experimental and analytical tools to unambiguously observe the atomically resolved chemical reactions. A great challenge of modern science has been to directly observe atomic motions during structural transitions, and while this was first achieved through a major advance in electron source brightness, the information content was still limited and new methods for image reconstruction using femtosecond electron diffraction methods were needed. One particular challenge lay in reconciling the innumerable possible nuclear configurations with the observation of chemical reaction mechanisms that reproducibly give the same kind of chemistry for large classes of molecules. The author shows that there is a simple solution that occurs during barrier crossing in which the highly anharmonic potential at that point in nuclear rearrangements couples high- and low-frequency vibrational modes to give highly localized nuclear motions, reducing hundreds of potential degrees of freedom to just a few key modes. Specific examples are given in this thesis, including two photoinduced phase transitions in an organic system, a ring closure reaction, and two direct observations of nuclear reorganization driven by spin transitions. The emerging field of structural dynamics promises to change the way we think about the physics of chemistry and this thesis provides tools to make it happen. |
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https://scigraph.springernature.com/ontologies/product-market-codes/P24009 |
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https://scigraph.springernature.com/ontologies/product-market-codes/C25007 |
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https://scigraph.springernature.com/ontologies/product-market-codes/C11006 |
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https://scigraph.springernature.com/ontologies/product-market-codes/P25056 |
| 773 0# - |
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Springer Nature eBook |
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Printed edition: |
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9783030548506 |
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Printed edition: |
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9783030548520 |
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Printed edition: |
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9783030548537 |
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Springer Theses, Recognizing Outstanding Ph.D. Research, |
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2190-5061 |
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ZDB-2-PHA |
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ZDB-2-SXP |
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Physics and Astronomy (SpringerNature-11651) |
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Physics and Astronomy (R0) (SpringerNature-43715) |
